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  • Templated synthesis of a large and flexible covalent porphyrinic cage bearing orthogonal recognition sites.

Templated synthesis of a large and flexible covalent porphyrinic cage bearing orthogonal recognition sites.

Chemical communications (Cambridge, England) (2012-04-21)
Julien Taesch, Valérie Heitz, Filip Topić, Kari Rissanen
ABSTRACT

A large covalent cage incorporating two porphyrins attached by four long and flexible polyether chains each bearing two 3-pyridyl ligands was synthesized from a DABCO-templated olefin metathesis reaction. The X-ray structure of the cage with the DABCO coordinated inside the cavity to the two zinc(II) porphyrins reveals a highly symmetric structure.

MATERIALS
Product Number
Brand
Product Description

Sigma-Aldrich
1,4-Diazabicyclo[2.2.2]octane, ReagentPlus®, ≥99%
Sigma-Aldrich
Dabco® 33-LV
Sigma-Aldrich
1,4-Diazabicyclo[2.2.2]octane, Vetec, reagent grade, 98%